posted on 2018-06-04, 14:53authored byMichael P. Barkley, Gonzalo González Abad, Thomas P. Kurosu, Robert Spurr, Sara Torbatian, Christophe Lerot
Using Ozone Monitoring Instrument (OMI) trace gas vertical column observations of nitrogen dioxide (NO2), formaldehyde (HCHO), sulfur dioxide (SO2), and glyoxal (CHOCHO), we have conducted a robust and detailed time series analysis to assess changes in local air quality for over 1000 locations (focussing on urban, oil refinery, oil port, and power plant targets) over the Middle East for 2005–2014. Apart from NO2, which is highest over urban locations, average tropospheric column levels of these trace gases are highest over oil ports and refineries. The highest average pollution levels over urban settlements are typically in Bahrain, Kuwait, Qatar, and the United Arab Emirates.
We detect 278 statistically significant and real linear NO2 trends in total. Over urban areas NO2 increased by up to 12 % yr−1, with only two locations showing a decreasing trend. Over oil refineries, oil ports, and power plants, NO2 increased by about 2–9 % yr−1. For HCHO, 70 significant and real trends were detected, with HCHO increasing by 2–7 % yr−1 over urban settlements and power plants and by about 2–4 % yr−1 over refineries and oil ports. Very few SO2 trends were detected, which varied in direction and magnitude (23 increasing and 9 decreasing). Apart from two locations where CHOCHO is decreasing, we find that glyoxal tropospheric column levels are not changing over the Middle East. Hence, for many locations in the Middle East, OMI observes a degradation in air quality over 2005–2014. This study therefore demonstrates the capability of OMI to generate long-term air-quality monitoring at local scales over this region.
Funding
This research used the ALICE and
SPECTRE High Performance Computing Facility at the
University of Leicester. We acknowledge the free use of
DOMINO tropospheric NO2 column data from www.temis.nl
and the HCHO and SO2 data from the NASA OMI portal
(http://disc.sci.gsfc.nasa.gov/Aura/data-holdings/OMI).
History
Citation
Atmospheric Chemistry and Physics, 2017, 17 (7), pp. 4687-4709
Author affiliation
/Organisation/COLLEGE OF SCIENCE AND ENGINEERING/Department of Physics and Astronomy
Version
VoR (Version of Record)
Published in
Atmospheric Chemistry and Physics
Publisher
European Geosciences Union (EGU), Copernicus Publications
All data products used in the analysis are freely
available online, apart from the OMI CHOCHO data which can be
accessed via C. Lerot (christophe.lerot@aeronomie.be). Please contact
the author for access to the time series analysis.
The Supplement related to this article is available online
at doi:10.5194/acp-17-4687-2017-supplement.