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Satellite quantification of methane emissions from South American countries: a high-resolution inversion of TROPOMI and GOSAT observations

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posted on 2025-03-07, 11:17 authored by Sarah E Hancock, Daniel J Jacob, Zichong Chen, Hannah Nesser, Aaron Davitt, Daniel J Varon, Melissa P Sulprizio, Nicholas Balasus, Lucas A Estrada, María Cazorla, Laura Dawidowski, Sebastián Diez, James D East, Elise Penn, Cynthia A Randles, John Worden, Ilse Aben, Robert ParkerRobert Parker, Joannes D Maasakkers
Abstract. We use 2021 TROPOMI and GOSAT satellite observations of atmospheric methane in an analytical inversion to quantify national methane emissions from South America at up to 25 km × 25 km resolution. From the inversion, we derive optimal posterior estimates of methane emissions, adjusting a combination of national anthropogenic emission inventories reported by individual countries to the United Nations Framework Convention on Climate Change (UNFCCC), the UNFCCC-based Global Fuel Exploitation Inventory (GFEIv2), and the Emissions Database for Global Atmospheric Research (EDGARv7) as prior estimates. We also evaluate two alternative wetland emission inventories (WetCHARTs and LPJ-wsl) as prior estimates. Our best posterior estimates for wetland emissions are consistent with previous inventories for the Amazon but lower for the Pantanal and higher for the Paraná. Our best posterior estimate of South American anthropogenic emissions is 48 (41–56) Tg a−1, where numbers in parentheses are the range from our inversion ensemble. This is 55 % higher than our prior estimate and is dominated by livestock (65 % of anthropogenic total). We find that TROPOMI and GOSAT observations can effectively optimize and separate national emissions by sector for 10 of the 13 countries and territories in the region, 7 of which account for 93 % of continental anthropogenic emissions: Brazil (19 (16–23) Tg a−1), Argentina (9.2 (7.9–11) Tg a−1), Venezuela (7.0 (5.5–9.9) Tg a−1), Colombia (5.0 (4.4–6.7) Tg a−1), Peru (2.4 (1.6–3.9) Tg a−1), Bolivia (0.96 (0.66–1.2) Tg a−1), and Paraguay (0.93 (0.88–1.0) Tg a−1). Our estimates align with the prior estimates for Brazil, Bolivia, and Paraguay but are significantly higher for other countries. Emissions in all countries are dominated by livestock (mainly enteric fermentation) except for oil–gas in Venezuela and landfills in Peru. Methane intensities from the oil–gas industry are high in Venezuela (33 %), Colombia (6.5 %), and Argentina (5.9 %). The livestock sector shows the largest difference between our top-down estimate and the UNFCCC prior estimates, and even countries using complex bottom-up methods report UNFCCC emissions significantly lower than our posterior estimate. These discrepancies could stem from underestimations in IPCC-recommended bottom-up calculations or uncertainties in the inversion from aggregation error and the prior spatial distribution of emissions.

Funding

Harvard University Climate Change Solutions Fund (CCSF)

NASA Carbon Monitoring System (CMS)

Graduate Research Fellowship Program (GRFP)

Directorate for Education & Human Resources

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International Methane Emissions Observatory (IMEO)

NASA ROSES grant no. 18-CMS18-0018

TerraFIRMA: Future Impacts Risks and Mitigation Actions

Natural Environment Research Council

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UK EO Climate Information Service (UKEO-CIS)

Natural Environment Research Council

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ESA GHG-CCI and Copernicus C3S projects (grant no. C3S2_312a_Lot2)

Amazonian Tall Tower Observatory (ATTO) for the measurement and long-term observation of climate-relevant trace gases as a basis for improved models for climate research

Federal Ministry of Education and Research

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Joint project ATTO: Pilot projects - Subproject 2: Effects of trace gases and aerosols on atmospheric chemistry and climate in the Central Amazon

Federal Ministry of Education and Research

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Brazilian Ministério da Ciência, Tecnologia e Inovação (MCTI/FINEP contract 01.11.01248.00)

History

Citation

Hancock, S. E., Jacob, D. J., Chen, Z., Nesser, H., Davitt, A., Varon, D. J., Sulprizio, M. P., Balasus, N., Estrada, L. A., Cazorla, M., Dawidowski, L., Diez, S., East, J. D., Penn, E., Randles, C. A., Worden, J., Aben, I., Parker, R. J., and Maasakkers, J. D.: Satellite quantification of methane emissions from South American countries: a high-resolution inversion of TROPOMI and GOSAT observations, Atmos. Chem. Phys., 25, 797–817, https://doi.org/10.5194/acp-25-797-2025, 2025.

Author affiliation

College of Science & Engineering Physics & Astronomy

Version

  • VoR (Version of Record)

Published in

Atmospheric Chemistry and Physics

Volume

25

Issue

2

Pagination

797 - 817

Publisher

Copernicus GmbH

issn

1680-7316

eissn

1680-7324

Acceptance date

2024-11-08

Copyright date

2025

Available date

2025-03-04

Language

en

Deposited by

Dr Robert Parker

Deposit date

2025-03-04

Data Access Statement

The blended TROPOMI + GOSAT satellite observations version 2 are available at https://registry.opendata.aws/blended-tropomi-gosat-methane (Balasus et al., 2023). The GOSAT methane retrievals version 9.0 are available at https://doi.org/10.5285/18ef8247f52a4cb6a14013f8235cc1eb (Parker and Boesch, 2020). Oil, gas, and coal emissions from the GFEIv2 inventory are available at https://doi.org/10.7910/DVN/HH4EUM (Scarpelli and Jacob, 2021). Methane emissions by sector from EDGARv7 are available at https://edgar.jrc.ec.europa.eu/dataset_ghg70 (Crippa et al., 2022). Wetland emissions from WetCHARTs v1.3.1 are available at https://doi.org/10.3334/ORNLDAAC/1915 (Bloom et al., 2024; Ma et al., 2021).

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